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Part of OC-08 — Amines & Diazonium Salts

Amines & Diazonium Salts: Visual Guide

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### Classification Table | Feature | 1° Amine | 2° Amine | 3° Amine | Quaternary Salt | |---|---|---|---|---| | Formula | $RNH_{2}$ | $R_{2}NH$ | $R_{3}N$ | $R_{4}N^{+}$ | | N–H bonds | 2 | 1 | 0 | 0 | | Basicity (aq) | 2nd | 1st (strongest) | 3rd | Not a base | | Gabriel? | Yes (aliphatic only) | No | No | No | | Carbylamine? | Yes (foul smell) | No | No | No | | Hinsberg (NaOH) | Soluble | Insoluble | No reaction | No reaction | ### Diazonium Reaction Map ``` $ArN_{2}^{+}$$Cl^{-}$ ├── + CuCl/HCl ────────────────→ ArCl [Sandmeyer] ├── + CuBr/HBr ────────────────→ ArBr [Sandmeyer] ├── + CuCN/KCN ────────────────→ ArCN [Sandmeyer] ├── + Cu°/HCl ─────────────────→ ArCl [Gattermann] ├── + $HBF_{4}$ →($\Delta$)─────────────→ ArF [Schiemann - ONLY ArF] ├── + $H_{3}PO_{2}$ ─────────────────→ ArH [Deamination] ├── + PhOH (alkaline) ────────→ orange-red azo dye └── + $PhNH_{2}$ (weak acid)──────→ yellow azo dye ``` ### Basicity Trend (Aqueous) | Compound | pKb (aq) | Relative Strength | |---|---|---| | ($CH_{3}$)_{2}NH (2°) | ≈ 3.27 | Strongest ↑ | | $CH_{3}$$NH_{2}$ (1°) | ≈ 3.38 | Strong | | ($CH_{3}$)_{3}N (3°) | ≈ 4.19 | Moderate | | $NH_{3}$ | ≈ 4.74 | Weak | | $C_{6}H_{5}$$NH_{2}$ (aniline) | ≈ 9.38 | Weakest ↓ | ### Aniline Resonance (SMILES: `Nc1ccccc1`) The lone pair on N enters the ring → partial positive charge on N in resonance structures → N is less available for protonation → weak base. `N(+)–C=C–C=C–C=C` (quinoid resonance form) ### Preparation Decision Tree ``` Want a PRIMARY ALIPHATIC amine? → Use Gabriel phthalimide (clean, no mixtures) → Or Nitro reduction (if Ar$NH_{2}$ is acceptable) → Or Hoffmann bromamide (but product has –1C) Want an AROMATIC AMINE (Ar$NH_{2}$)? → Use Nitro reduction ONLY (Gabriel won't work) Want FEWER CARBONS in the product? → Use Hoffmann bromamide (–1C vs starting amide) ```$

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