Part of OC-08 — Amines & Diazonium Salts

Amines & Diazonium Salts: Visual Guide

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Classification Table

Feature1° Amine2° Amine3° AmineQuaternary Salt
FormulaRNH2RNH_{2}R2NHR_{2}NHR3NR_{3}NR4N+R_{4}N^{+}
N–H bonds2100
Basicity (aq)2nd1st (strongest)3rdNot a base
Gabriel?Yes (aliphatic only)NoNoNo
Carbylamine?Yes (foul smell)NoNoNo
Hinsberg (NaOH)SolubleInsolubleNo reactionNo reaction

Diazonium Reaction Map

$ArN_{2}^{+}$$Cl^{-}$
  ├── + CuCl/HCl ────────────────→ ArCl    [Sandmeyer]
  ├── + CuBr/HBr ────────────────→ ArBr    [Sandmeyer]
  ├── + CuCN/KCN ────────────────→ ArCN    [Sandmeyer]
  ├── + Cu°/HCl ─────────────────→ ArCl    [Gattermann]
  ├── + $HBF_{4}$ →($\Delta$)─────────────→ ArF     [Schiemann - ONLY ArF]
  ├── + $H_{3}PO_{2}$ ─────────────────→ ArH     [Deamination]
  ├── + PhOH (alkaline) ────────→ orange-red azo dye
  └── + $PhNH_{2}$ (weak acid)──────→ yellow azo dye

Basicity Trend (Aqueous)

CompoundpKb (aq)Relative Strength
(CH3CH_{3})_{2}NH (2°)≈ 3.27Strongest ↑
CH_{3}$$NH_{2} (1°)≈ 3.38Strong
(CH3CH_{3})_{3}N (3°)≈ 4.19Moderate
NH3NH_{3}≈ 4.74Weak
C_{6}H_{5}$$NH_{2} (aniline)≈ 9.38Weakest ↓

Aniline Resonance (SMILES: Nc1ccccc1)

The lone pair on N enters the ring → partial positive charge on N in resonance structures → N is less available for protonation → weak base.

N(+)–C=C–C=C–C=C (quinoid resonance form)

Preparation Decision Tree

Want a PRIMARY ALIPHATIC amine?
  → Use Gabriel phthalimide (clean, no mixtures)
  → Or Nitro reduction (if Ar$NH_{2}$ is acceptable)
  → Or Hoffmann bromamide (but product has –1C)

Want an AROMATIC AMINE (Ar$NH_{2}$)?
  → Use Nitro reduction ONLY (Gabriel won't work)

Want FEWER CARBONS in the product?
  → Use Hoffmann bromamide (–1C vs starting amide)

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